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Phonon induced line broadening and population of the dark exciton in a deeply trapped localized emitter in monolayer WSe2

机译:声子在单层WSe 2 中深陷的局域发射极中引起声子扩宽和暗激子的分布

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摘要

We study trapped single excitons in a monolayer semiconductorwith respect to their temperature stability, spectral diffusion and decaydynamics. In a mechanically exfoliated WSe2 sheet, we could identifydiscrete emission features with emission energies down to 1.516 eV whichare spectrally isolated in a free spectral range up to 80 meV. The strongspectral isolation of our localized emitter allow us to identify strongsignatures of phonon induced spectral broadening for elevated temperaturesaccompanied by temperature induced luminescence quenching. A directcorrelation between the droop in intensity at higher temperatures with thephonon induced population of dark states in WSe is established. While ourexperiment suggests that the applicability of monolayered quantum emittersas coherent single photon sources at elevated temperatures may be limited,the capability to operate them below the GaAs band-edge makes themhighly interesting for GaAs-monolayer hybrid quantum photonic structures.
机译:我们研究了单层半导体中捕获的单激子的温度稳定性,光谱扩散和衰减动力学。在机械剥离的WSe2薄片中,我们可以识别出发射能量低至1.516 eV的离散发射特征,这些特征在高达80 meV的自由光谱范围内被光谱隔离。局部发射体的强光谱隔离使我们能够识别声子引起的光谱增宽的强信号,该现象由温度引起的发光猝灭伴随着升高的温度。建立了在较高温度下的强度下降与声子诱导的WSe中黑暗状态种群之间的直接相关性。尽管我们的实验表明,单层量子发射器在高温下作为相干单光子源的适用性可能受到限制,但在GaAs频带边缘以下操作它们的能力使它们对于GaAs-单层混合量子光子结构非常感兴趣。

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